Coherent Raman Spectroscopy -  G. L. Eesley

Coherent Raman Spectroscopy (eBook)

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2013 | 1. Auflage
152 Seiten
Elsevier Science (Verlag)
978-1-4831-5391-9 (ISBN)
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Coherent Raman Spectroscopy provides a unified and general account of the fundamental aspects of nonlinear Raman spectroscopy, also known as coherent Raman spectroscopy. The theoretical basis from which coherent Raman spectroscopy developed is described, along with its applications, utility, and implementation as well as advantages and disadvantages. Experimental data which typifies each technique is presented. This book is comprised of four chapters and opens with an overview of nonlinear optics and coherent Raman spectroscopy, followed by a discussion on nonlinear transfer function of matter. The derivation of third-order nonlinear effects is described and the problem is specialized to one dimension by assuming monochromatic plane waves propagating in the z direction. The next chapter reviews the salient features of seven coherent Raman techniques by calculating the resonant and non-resonant signal contributions in the monochromatic plane wave limit. Finally, the general areas of application of coherent Raman spectroscopy are highlighted. This monograph is written primarily for uninitiated or endeavoring coherent Raman spectroscopists and should also be of interest to experienced industrial and academic researchers.
Coherent Raman Spectroscopy provides a unified and general account of the fundamental aspects of nonlinear Raman spectroscopy, also known as coherent Raman spectroscopy. The theoretical basis from which coherent Raman spectroscopy developed is described, along with its applications, utility, and implementation as well as advantages and disadvantages. Experimental data which typifies each technique is presented. This book is comprised of four chapters and opens with an overview of nonlinear optics and coherent Raman spectroscopy, followed by a discussion on nonlinear transfer function of matter. The derivation of third-order nonlinear effects is described and the problem is specialized to one dimension by assuming monochromatic plane waves propagating in the z direction. The next chapter reviews the salient features of seven coherent Raman techniques by calculating the resonant and non-resonant signal contributions in the monochromatic plane wave limit. Finally, the general areas of application of coherent Raman spectroscopy are highlighted. This monograph is written primarily for uninitiated or endeavoring coherent Raman spectroscopists and should also be of interest to experienced industrial and academic researchers.

Front Cover 1
Coherent Raman Spectroscopy 4
Copyright Page 5
Table of Contents 10
Dedication 6
Preface 8
Chapter 1. INTRODUCTION 12
A. Nonlinear Optics and Coherent Raman Spectroscopy 12
B. Objectives 16
C. Notation and Conventions 17
Chapter 2. NONLINEAR TRANSFER FUNCTION OF MATTER 18
A. Derivation of Third-Order Nonlinear Effects 18
B. Semiclassical Coupling to Maxwell's Equations 28
C. Additional Symmetry Considerations 34
Chapter 3. COHERENT RAMAN TECHNIQUES 35
A. Signals of Various Techniques 35
B. Noises of Various Techniques 69
C. Comparison of Techniques 83
Chapter 4. APPLICATIONS 90
A. Introductory Remarks 90
B. General Areas of Application 91
C. Selected Results and Bibliographies 92
Appendix 1: PROBABILITY FOR NONDISSIPATIVE INTERACTIONS 119
Appendix 2: THIRD-ORDER NONLINEAR SUSCEPTIBILITY 123
Appendix 3: NONLINEAR FIELD GENERATION BY QUASIMONOCHROMATIC FIELDS 129
Appendix 4: CALCULATION OF SIGNAL-TO-NOISE RATIOS FROM THE OPTICAL POWER SPECTRAL DENSITIES 132
Appendix 5: RIKE SIGNAL FIELD SPATIAL PROFILE, POWER AND HETERODYNING EFFICIENCY 136
Appendix 6: RELATIONSHIP OF X(3)TO THE RAMAN SCATTERING CROSS SECTION 142
Appendix 7: PHYSICAL CONSTANTS AND X(3) (CGS-ESU).X(3) (MKS) CONVERSION 145
REFERENCES 146
INDEX 151

Erscheint lt. Verlag 22.10.2013
Sprache englisch
Themenwelt Naturwissenschaften Physik / Astronomie Optik
Technik
ISBN-10 1-4831-5391-6 / 1483153916
ISBN-13 978-1-4831-5391-9 / 9781483153919
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